ISSN 1008-5548

CN 37-1316/TU

Last Issue

Preparation technology of coated particles for nuclear fuel in high-temperature gas-cooled reactors

GAO Ming1 ,LU Zhenming2,3,LU Anyuan3 ,YU Deshui1 ,ZHAO Yongqian1 ,GAO Tian3 ,LIU Bing2

1. China North Nuclear Fuel Co. , Ltd. , Baotou 014035, China;

2. Institute of Nuclear and New Energy Technology, Tsinghua University, Beijing 100084, China;

3. Hubei Key Laboratory of Coal Conversion and New Carbon Materials, School of Chemistry and Chemical Engineering,Wuhan University of Science and Technology, Wuhan 430081, China

Abstract

Significance The fuel elements used in pebble-bed high-temperature gas-cooled reactors (PB-HTRs) are graphite spheres containing thousands of Tri-structural isotropic (TRISO) coated particles, which are fabricated through quasi-isostatic pressing. The coating layer of the coated particles serves as the first barrier to guarantee reactor safety. Before fuel element compression, a compression buffer layer, composed of the same material as the matrix, is wrapped around the surface of the coated particles. This layer directly and effectively mitigates damage to the coating layer during the element production process, a step known as the overcoating process.

Progress China’s high-temperature gas-cooled reactors (HTRs) have evolved over more than four decades, from the 10 MW high-temperature gas-cooled reactor-test module (HTR-10) to the 200 MW high-temperature gas-cooled reactor pebble-bed module (HTR-PM). Correspondingly, overcoating technologies, a crucial part of nuclear fuel production, have progressed through multiple stages: basic research-level, laboratory-scale, pilot-scale, commercial demonstration, and commercialization. In terms of equipment structure, various types of overcoating equipment have been developed, including laboratory-scale onion-shaped and truncated-cone-shaped types, a meshed drum-type for commercial demonstration, and non-porous-drum and planetary types for large-scale commercial applications. The single-batch capacity has increased significantly, from 1 kgU to tens of kilograms. Meanwhile, the automation level, safety, and environmental friendliness of the equipment have been progressively improved while ensuring high product yield and quality. Advanced research methods, such as online analysis of particle shape and size, and numerical simulation, are used in equipment design, development, and process optimization, effectively accelerating progress and enhancing the effectiveness of research and development. So far, China's nuclear fuel overcoating technology has surpassed its international counterparts in productivity, product quality, and equipment automation and advancement through decades of dedicated efforts by several generations of R&D personnel.

Prospects The evolution and advancement of nuclear fuel preparation technology, along with the scientific challenges in engineering, will garner increasing attention and attract professionals from diverse research domains into this field. Disciplines and research fields, including materials science, particle kinetic theory, fluid mechanics, and numerical simulation, will converge and give rise to new interdisciplinary directions in the study of the overcoating process. Theoretical achievements will also lead to novel engineering concepts, promoting innovation and upgrading of overcoating equipment. With the widespread adoption of computer technology, advancements in image technology, enhanced precision and capabilities of detection instruments, and ongoing process refinement and optimization, process control technology will be extensively applied to the overcoating process. This will significantly enhance the automation level of overcoating equipment. Artificial intelligence (AI) is also set to be deeply integrated into the industrial production of overcoating particles. By combining human expertise and the computer's analytical capabilities, AI will facilitate decision-making and task execution through big data analysis. The immediate result of incorporating AI lies in the optimization of process parameters, thereby achieving optimal product quality and stability.

Conclusions With intensified theoretical research, improved automation, and the integration of artificial intelligence, overcoating technology will undergo multidimensional technological transformations and evolve towards a more efficient, automated, and intelligent direction. TRISO-coated particles have played a pivotal role in ensuring the inherent safety of HTRs, making their structure highly favored for various types of nuclear reactors. With the rapid development of HTRs and increasing safety demands for reactors, the demand for accident-tolerant nuclear fuel incorporating TRISO particles will surge substantially. Consequently, overcoating technology is poised to have broader application prospects.

Keywords:high-temperature gas-cooled reactor; spherical nuclear fuel element; overcoating technology; overcoating particle

Get Citation:GAO Ming, LU Zhenming, LU Anyuan, et al. Preparation technology of coated particles for nuclear fuel in high-temperature gas-cooled reactors[J]. China Powder Science and Technology,2025,31(5):1−11.

Received: 2024-11-29 .Revised: 2025-05-21,Online: 2025-06-27

Funding Project:国家自然科学基金项目,编号:22403072;国家科技重大专项项目,编号:ZX06901。

First Author:高明(1983—),男,高级工程师,硕士,研究方向为高温气冷堆球形燃料元件制造。E-mail:gwkj-jsk@cnnfc202. com。

Corresponding Author:卢振明(1975—),男,教授,博士,硕士生导师,研究方向为核燃料材料及球形颗粒制备。E-mail:luzhenming@wust. edu. cn。

DOI:10.13732/j.issn.1008-5548.2025.05.007

CLC No:TL352.2;TB4             Type Code: A

Serial No:1008-5548(2025)05-0001-11